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Region-gridding recycling of bulk organic waste: Emerging views based on coordinated urban and rural

Wenbing Tan, Dongyu Cui, Xiaohui Zhang, Beidou Xi

《环境科学与工程前沿(英文)》 2020年 第14卷 第6期 doi: 10.1007/s11783-020-1291-4

摘要: Abstract Bulk organic waste (BOW) has a large output in China. The improper disposal of BOW will not only bring serious environmental pollution, but also cause waste of biomass resources. The viewpoint proposes a region-gridding recycling management system of BOW that highlights the coordinated development of environmental, agricultural and energy elements in urban and rural areas. The viewpoint aims to drive the upstream and downstream industrial chains of BOW treatments, avoid the repeated construction of resource facilities, guide the upgrading of resource-based technologies, promote the professionalization of farmers, and thus built the high-quality modern agricultural recycling industrial park based on system management.

关键词: Bulk organic waste     Recycling     Urban-rural coordination     Management system    

Environmental effects and risk control of antibiotic resistance genes in the organic solid waste aerobic

《环境科学与工程前沿(英文)》 2021年 第15卷 第6期 doi: 10.1007/s11783-021-1415-5

摘要:

• ARGs were detected in livestock manure, sludge, food waste and fermentation dregs.

关键词: Antibiotic resistance genes     Organic solid waste     Aerobic composting     Livestock manure     Sludge    

Developing “precise-acting” strategies for improving anaerobic methanogenesis of organic waste: Insights

《环境科学与工程前沿(英文)》 2022年 第16卷 第6期 doi: 10.1007/s11783-021-1508-1

摘要: Methanogenesis is the last step in anaerobic digestion, which is usually a rate-limiting step in the biological treatment of organic waste. The low methanogenesis efficiency (low methane production rate, low methane yield, low methane content) substantially limits the development of anaerobic digestion technology. Traditional pretreatment methods and bio-stimulation strategies have impacts on the entire anaerobic system and cannot directly enhance methanogenesis in a targeted manner, which was defined as “broad-acting” strategies in this perspective. Further, we discussed our opinion of methanogenesis process with insights from the electron transfer system of syntrophic partners and provided potential targeted enhancing strategy for high-efficiency electron transfer system. These “precise-acting” strategies are expected to achieve an efficient methanogenesis process and enhance the bio-energy recovery of organic waste.

关键词: Methanogenesis     Anaerobic digestion     Enhancing strategy     Electron transfer     Organic waste    

Synthesis of porous carbon from orange peel waste for effective volatile organic compounds adsorption

《化学科学与工程前沿(英文)》 2023年 第17卷 第7期   页码 942-953 doi: 10.1007/s11705-022-2264-x

摘要: Volatile organic compounds have posed a serious threat to the environment and human health, which require urgent and effective removal. In recent years, the preparation of porous carbon from biomass waste for volatile organic compounds adsorption has attracted increasing attention as a very cost-effective and promising technology. In this study, porous carbon was synthesized from orange peel by urea-assisted hydrothermal carbonization and KOH activation. The role of typical components (cellulose, hemicellulose, and lignin) in pore development and volatile organic compounds adsorption was investigated. Among the three components, hemicellulose was the major contributor to high porosity and abundant micropores in porous carbon. Higher hemicellulose content led to more abundant –COOR, amine-N, and pyrrolic/pyridonic-N in the derived hydrochar, which were favorable for porosity formation during activation. In this case, the toluene adsorption capacity of the porous carbon improved from 382.8 to 485.3 mg·g–1. Unlike hemicellulose, cellulose reduced the >C=O, amine-N, and pyrrolic/pyridonic-N content of the hydrochar, which caused porosity deterioration and worse toluene adsorption performance. Lignin bestowed the hydrochar with slightly increased –COOR, pyrrolic/pyridonic-N, and graphitic-N, and reduced >C=O, resulting in comparatively poor porosity and more abundant micropores. In general, the obtained porous carbon possessed abundant micropores and high specific surface area, with the highest up to 2882 m2·g–1. This study can provide guidance for selecting suitable biomass waste to synthesize porous carbon with better porosity for efficient volatile organic compounds adsorption.

关键词: biomass waste     porous carbon     feedstock composition     urea-assisted hydrothermal carbonization     toluene adsorption     N-doped hydrochar    

In vitro agonistic and antagonistic endocrine disrupting effects of organic extracts from waste water

Kaifeng RAO, Na LI, Mei MA, Zijian WANG

《环境科学与工程前沿(英文)》 2014年 第8卷 第1期   页码 69-78 doi: 10.1007/s11783-013-0502-7

摘要: Effluents from wastewater treatment plant (WWTP) have been reported to have a broad spectrum of endocrine disrupting compounds (EDCs). The majority of studies have focused on the occurrence of estrogenic activity, while ignoring nuclear hormone receptors (NRs) pathways. In the present study, a battery of in vitro yeast bioassays and a cell bioassay, including antagonistic and agonistic effects on estrogen receptor (ER), androgen receptor (AR), progesterone receptor (PR), estrogen-related receptor (ERR) and aryl hydrocarbon receptor (AHR), were conducted to evaluate the removal efficiencies of EDCs by different treatment processes of a WWTP located in Beijing. Estrogenic, anti-estrogenic, anti- androgenic, anti-progesteronic, anti-ERR and the activation of AHR activities were detected in samples from all treatment processes and the receiving water. The concentration of estrogenic contaminants with estradiol (E ) equivalent concentrations ranged from 0.82 × 10 to 3.54 × 10 g E -EQ·L . The concentration of anti-estrogenic contaminants with 4-hydroxytamoxifen (4-OHT) equivalent concentrations ranged from 1.24 × 10 to 2.36 × 10 g 4-OHT-EQ·L . The concentration of anti-androgenic contaminants ranged from 2.21 × 10 to 3.52 × 10 g flutamide-EQ·L . The concentration of anti-progesteronic contaminants ranged from 3.15 × 10 to 2.71 × 10 g RU486-EQ·L . The concentration of anti-ERR contaminants ranged from 7.09 × 10 to 6.50 × 10 g 4-OHT-EQ·L . The concentration of AHR activators ranged from 1.7 × 10 to 3.4 × 10 g TCDD-EQ·L . These processes including secondary clarifier, coagulation, as well as coal and sand filtration could eliminated 67.2% of estrogenic contaminants, 47.0% of anti-estrogenic contaminants, 98.3% of anti-androgenic contaminants, 88.4% of anti-progesteronic contaminants, 65.4% of anti-ERR contaminants and 46.9% of AHR activators. WWTP effluents contain multiple receptor disruptors may have very complex adverse effects on exposed organisms.

关键词: waste water     in vitro     recombinant yeast assay     ethoxyresorufin-O-deethylase (EROD)     receptor     endocrine    

Optimizing iodine capture performance by metal–organic framework containing with bipyridine units

《化学科学与工程前沿(英文)》 2023年 第17卷 第4期   页码 395-403 doi: 10.1007/s11705-022-2218-3

摘要: Radioactive iodine exhibits medical values in radiology, but its excessive emissions can cause environmental pollution. Thus, the capture of radioiodine poses significant engineering for the environment and medical radiology. The adsorptive capture of radioactive iodine by metal–organic frameworks (MOFs) has risen to prominence. In this work, a Th-based MOF (denoted as Th-BPYDC) was structurally designed and synthesized, consisting of [Th63-O)43-OH)4(H2O)6]12+ clusters, abundant bipyridine units, and large cavities that allowed guest molecules diffusion and transmission. Th-BPYDC exhibited the uptake capacities of 2.23 g·g−1 and 312.18 mg·g−1 towards I2 vapor and I2 dissolved in cyclohexane, respectively, surpassing its corresponding analogue Th-UiO-67. The bipyridine units boosted the adsorption performance, and Th-BPYDC showed good reusability with high stability. Our work thus opened a new way for the synthesis of MOFs to capture radioactive iodine.

关键词: metal–organic framework     iodine     adsorption     nuclear waste     environmental remediation    

E-waste environmental contamination and harm to public health in China

null

《医学前沿(英文)》 2015年 第9卷 第2期   页码 220-228 doi: 10.1007/s11684-015-0391-1

摘要:

The adverse effects of electronic waste (e-waste) on the human body have stirred up concern in recent years. China is one of the countries that confront serious pollution and human exposure of e-waste, and the majority of the population is exposed to potentially hazardous substances that are derived from informal e-waste recycling processes. This study reviews recent reports on human exposure to e-waste in China, with particular focus on exposure routes (e.g., inhalation and ingestion) and several toxicities of human (e.g., endocrine system, respiratory system, reproductive system, developmental toxicity, neurotoxicity, and genetic toxicity). Pieces of evidence that associate e-waste exposure with human health effects in China are assessed. The role of toxic heavy metals (e.g., lead, cadmium, chromium, mercury, and nickel) and organic pollutants (e.g., polybrominated diphenyl ethers (PBDEs), polychlorinated biphenyl (PCBs), polycyclic aromatic hydrocarbons (PAHs), polybrominated biphenyls (PBBs), polyhalogenated aromatic hydrocarbons (PHAHs), bisphenol A (BPA)) on human health is also briefly discussed.

关键词: e-waste     heavy metal     organic pollutant     hazardous     toxicity     human health     China    

大块非晶合金:历史发展和当前研究 Review

Akihisa Inoue

《工程(英文)》 2015年 第1卷 第2期   页码 185-191 doi: 10.15302/J-ENG-2015038

摘要:

通过关注采用传统模型铸造方法合成首批大块非晶合金的触发点,本文论述了大块非晶合金的当前研究进展情况。该综述涵盖大块非晶合金的背景、发现、特点和应用以及近期与其相关的研究主题。由于其性质独特,非晶形成能力高且成本低廉,大块非晶合金 ( 尤其是铁基大块非晶合金) 的应用范围正逐步扩大。在不久的将来,大块非晶合金在工程领域的重要性预计将稳步提高,预期将上述创新型金属材料用于基础科学研究的热度仍将持续。

关键词: 大块非晶合金,模型铸造,金属材料,结构弛豫    

Removal of odors and VOCs in municipal solid waste comprehensive treatment plants using a novel three-stage

《环境科学与工程前沿(英文)》 2021年 第15卷 第3期 doi: 10.1007/s11783-021-1421-7

摘要:

A novel three-stage integrated biofilter (TSIBF) composed of acidophilic bacteria reaction segment (ABRS), fungal reaction segment (FRS) and heterotrophic bacteria reaction segment (HBRS) was constructed for the treatment of odors and volatile organic compounds (VOCs)from municipal solid waste (MSW) comprehensive treatment plants. The performance, counts of predominant microorganisms, and bioaerosol emissions of a full-scale TSIBF system were studied. High and stable removal efficiencies of hydrogen sulfide, ammonia and VOCs could be achieved with the TSIBF system, and the emissions of culturable heterotrophic bacteria, fungi and acidophilic sulfur bacteria were relatively low.

关键词: Biofiltration     Multi-stage biofilter     Volatile organic compounds     Waste gas treatment     Bioaerosol emissions    

Anaerobic treatment of fresh leachate from a municipal solid waste incinerator by upflow blanket filter

Pinjing HE, Min LI, Suyun XU, Liming SHAO,

《环境科学与工程前沿(英文)》 2009年 第3卷 第4期   页码 404-411 doi: 10.1007/s11783-009-0149-6

摘要: This paper describes the feasibility of fresh leachate treatment by an upflow blanket filter (UBF). Through dilution and partial effluent recycling, the organic loading rates increased from 0.51to 14.56kg COD/(m·d), meanwhile the corresponding hydraulic retention time decreased from 9.0d to 3.6d. The reactor was able to achieve steady-state within 80d. Based on the distribution of COD fluxes in the process, it was concluded that anabolism was the main pathway of COD removal in the initial phase (1―33d), accounting for 57%―85% of total COD removed. As the anaerobic consortium of bacteria reached steady-state (after 70―86d), the majority of COD removed was transformed into methane, because the specific methane yield was close to the theoretical value (0.36L CH/(g COD)).

关键词: distribution of COD fluxes     effluent recycling     leachate     methane yield     organic loading rate     upflow blanket filter    

Changes in bulk soil affect the disease-suppressive rhizosphere microbiome against Fusarium wilt disease

Lin FU, Wu XIONG, Francisco DINI-ANDREOTE, Beibei WANG, Chengyuan TAO, Yunze RUAN, Zongzhuan SHEN, Rong LI, Qirong SHEN

《农业科学与工程前沿(英文)》 2020年 第7卷 第3期   页码 307-316 doi: 10.15302/J-FASE-2020328

摘要:

Harnessing disease-suppressive microbiomes constitutes a promising strategy for optimizing plant growth. However, relatively little information is available about the relationship between bulk and rhizosphere soil microbiomes. Here, the assembly of banana bulk soil and rhizosphere microbiomes was investigated in a monoculture system consisting of bio-organic (BIO) and organic management practices. Applying BIO practice in newly reclaimed fields resulted in a high-efficiency biocontrol rate, thus providing a promising strategy for pre-control of Fusarium wilt disease. The soil microbiota was further characterized by MiSeq sequencing and quantitative PCR. The results indicate that disease suppression was mediated by the structure of a suppressive rhizosphere microbiome with respect to distinct community composition, diversity and abundance. Overall microbiome suppressiveness was primarily related to a particular set of enriched bacterial taxa affiliated with s, , , , and . Finally, structural equation modeling was used to show that the changes in bulk soil bacterial community determined its induced rhizosphere bacterial community, which serves as an important and direct factor in restraining the pathogen. Collectively, this study provides an integrative approach to disentangle the biological basis of disease-suppressive microbiomes in the context of agricultural practice and soil management.

关键词: agricultural practice     bulk soil     disease suppression     rhizosphere ecology    

Synthesis and bulk polymerization kinetics of monomer dehydroabietic acid-(2-acryloyloxy-ethoxy)-ethyl

Haibo ZHANG,Yanping YANG,He LIU,Jie SONG,Shibin SHANG,Zhanqian SONG

《农业科学与工程前沿(英文)》 2017年 第4卷 第1期   页码 97-105 doi: 10.15302/J-FASE-2016115

摘要: A bulk polymerization monomer dehydro- abietic acid-(2-acryloyloxy-ethoxy)-ethyl ester (DHA-DG-AC) was synthesized from dehydroabietic acid (DHA). The chemical structure of DHA-DG-AC was characterized by H NMR, C NMR, MS and FT-IR. The kinetics of the bulk polymerization of DHA-DG-AC was investigated by Differential Scanning Calorimeter (DSC). Two kinds of kinetic model (nth-order model and autocatalytic model) were used to investigate the polymerization process. The results showed that the experimental DSC curves were consistent with the computational data generated by the autocatalytic kinetic model, and the value of was 95.73 kJ·mol .

关键词: dehydroabietic acid     bulk polymerization     kinetics     autocatalytic kinetic model    

含高浓度无机颗粒的有机废液分离及回用技术 Article

汪华林, 付鹏波, 李剑平, 黄渊, 赵颖, 姜来, 方向晨, 杨涛, 黄朝晖, 黄诚

《工程(英文)》 2018年 第4卷 第3期   页码 406-415 doi: 10.1016/j.eng.2018.05.014

摘要:

有机废液的无害化、资源化处理是环境工程的前沿之一,随着化学品需求不断增加,石油、煤和天然气转化中排放的含高浓度无机污染物的有机废液问题更趋严重。本文通过同步高速摄像技术发现了三维旋转湍流场中颗粒物高速自转和翻转现象,自转速度高达2000~6000 rad·s-1,利用这一现象发明了颗粒物孔隙中有机物旋流自转脱除方法,开发了废液中有机污染物旋流自转回收、无机颗粒物气流加速度分级回用的工艺流程,并成功应用于中国石化第一套自主研发的沸腾床渣油加氢工程示范装置中。该技术与美国T-STAR含废催化剂的有机废液固定床气提技术相比,同温度下催化剂颗粒脱液效率最高可提高44.9个百分点,实现95%脱液效率的处理时间从1956.5 s降低到8.4 s,并实现了外排催化剂颗粒按活性分级进行回用。提出了200万吨/年沸腾床渣油加氢装置的外排有机废液控制及无机颗粒回收利用技术方案,预期可回收柴油3100吨/年,高活性催化剂颗粒647吨/年,降低装置新鲜催化剂消耗量518吨/年,直接经济效益3728万元/年,具有显著的经济、社会和环境效益。

关键词: 有机废液     无机颗粒     旋流脱液     颗粒自转     气流加速度分选    

Effect of the addition of organic carbon sources on nitrous oxide emission in anaerobic-aerobic (low

Hongjing LI, Xiurong CHEN, Yinguang CHEN

《环境科学与工程前沿(英文)》 2010年 第4卷 第4期   页码 490-499 doi: 10.1007/s11783-010-0248-4

摘要: The effect of additional organic carbon sources on the production of nitrous oxide (N O) in anaerobic-aerobic (low dissolved oxygen) real wastewater treatment system was investigated. In this paper, three laboratory-scale sequencing batch reactors (SBRs) (SBR-1, SBR-2 and SBR-3) were operating under an anaerobic-aerobic (low dissolved oxygen, 0.15–0.45 mg·L ) configuration. The SBRs were ‘long-term cultured’ respectively with a single municipal wastewater sample, sodium acetate, and a waste-activated sludge alkaline fermentation liquid as the additional carbon sources of real wastewater. Off-gas analysis showed that N O was emitted into the atmosphere during the aerobic (low dissolved oxygen) period in the three SBRs, and the order of N O emission rate was SBR-2>SBR-1>SBR-3. It was observed that the higher poly-β-hydroxyvalerate fraction of polyhydroxyalkanoates, the lower glycogen transformation and less nitrite accumulation was in SBR-3, while the opposite behavior was observed in SBR-2. Further research indicated that the interaction of the factors above potentially affected the N O emission in the anaerobic-aerobic (low dissolved oxygen) system.

关键词: anaerobic-aerobic (low dissolved oxygen)     nitrous oxide (N2O) emitting rate     municipal wastewater     waste activated sludge     alkaline fermentation liquid    

用于微电子机械系统封装的体硅键合技术和薄膜密封技术

王渭源,王跃林

《中国工程科学》 2002年 第4卷 第6期   页码 56-62

摘要:

对静电键合、体硅直接键合和界面层辅助键合等三种体硅键合技术,整片操作、局部操作和选择保护等三种密封技术,以及这些技术用于微电子机械系统的密封作了评述,强调在器件研究开始时应考虑封装问题,具体技术则应在保证器件功能和尽量减少芯片复杂性两者之间权衡决定。

关键词: 体硅键合技术     薄膜密封技术     微电子机械系统封装技术    

标题 作者 时间 类型 操作

Region-gridding recycling of bulk organic waste: Emerging views based on coordinated urban and rural

Wenbing Tan, Dongyu Cui, Xiaohui Zhang, Beidou Xi

期刊论文

Environmental effects and risk control of antibiotic resistance genes in the organic solid waste aerobic

期刊论文

Developing “precise-acting” strategies for improving anaerobic methanogenesis of organic waste: Insights

期刊论文

Synthesis of porous carbon from orange peel waste for effective volatile organic compounds adsorption

期刊论文

In vitro agonistic and antagonistic endocrine disrupting effects of organic extracts from waste water

Kaifeng RAO, Na LI, Mei MA, Zijian WANG

期刊论文

Optimizing iodine capture performance by metal–organic framework containing with bipyridine units

期刊论文

E-waste environmental contamination and harm to public health in China

null

期刊论文

大块非晶合金:历史发展和当前研究

Akihisa Inoue

期刊论文

Removal of odors and VOCs in municipal solid waste comprehensive treatment plants using a novel three-stage

期刊论文

Anaerobic treatment of fresh leachate from a municipal solid waste incinerator by upflow blanket filter

Pinjing HE, Min LI, Suyun XU, Liming SHAO,

期刊论文

Changes in bulk soil affect the disease-suppressive rhizosphere microbiome against Fusarium wilt disease

Lin FU, Wu XIONG, Francisco DINI-ANDREOTE, Beibei WANG, Chengyuan TAO, Yunze RUAN, Zongzhuan SHEN, Rong LI, Qirong SHEN

期刊论文

Synthesis and bulk polymerization kinetics of monomer dehydroabietic acid-(2-acryloyloxy-ethoxy)-ethyl

Haibo ZHANG,Yanping YANG,He LIU,Jie SONG,Shibin SHANG,Zhanqian SONG

期刊论文

含高浓度无机颗粒的有机废液分离及回用技术

汪华林, 付鹏波, 李剑平, 黄渊, 赵颖, 姜来, 方向晨, 杨涛, 黄朝晖, 黄诚

期刊论文

Effect of the addition of organic carbon sources on nitrous oxide emission in anaerobic-aerobic (low

Hongjing LI, Xiurong CHEN, Yinguang CHEN

期刊论文

用于微电子机械系统封装的体硅键合技术和薄膜密封技术

王渭源,王跃林

期刊论文